If I remember right, given that free neutrons aren’t stable and have a very short half life, it would be explosively unwise even if it was physically possible.

Yes, a free neutron decays to a proton, an electron and an electron neutrino with a half life of 879 seconds. This decay releases 0.8MeV of energy (mostly in the form of kinetic energy of the electron).

My back of the envelope calculation shows that 1 gram of neutronium (approximately a mole) will release 43MW of energy continuously. Multiply that by 10^14 (the number of grams of neutronium per teaspoon) and the resultant energy release would be unimaginably huge. 'Explosively' does not even begin to describe it.